Relevance of radon progeny measurements for the assessment of inhalation doses in groundwater utilities.

The high radon concentrations measured in the indoor air of groundwater facilities and the prevalence of the problem have been known for several years. Unlike in other workplaces, in groundwater plants, radon is released into the air from the water treatment processes. During the measurements of this study, the average radon concentrations varied from 500 to 8800 Bq m-3. In addition, the indoor air of the treatment plants is filtered and there are no significant internal aerosol sources. However, only a few published studies on groundwater plants have investigated the properties of the radon progeny aerosol, such as the equilibrium factor (F) or the size distribution of the aerosol, which are important for assessing the dose received by workers. Moreover, the International Commission on Radiological Protection has not provided generic aerosol parameter values for dose assessment in groundwater treatment facilities. In this study, radon and radon progeny measurements were carried out at three groundwater plants. The results indicate surprisingly high unattached fractions (fp= 0.27-0.58), suggesting a low aerosol concentration in indoor air. The correspondingFvalues were 0.09-0.42, well below those measured in previous studies. Based on a comparison of the effective dose rate calculations, either the determination of thefpor, with certain limitations, the measurement of radon is recommended. Dose rate calculation based on the potential alpha energy concentration alone proved unreliable.

Radon Exposure Concentrations in Finnish Workplaces.

ABSTRACT: The aim of this study was to obtain information on the radon concentrations to which Finnish workers are exposed. Radon measurements were conducted as integrated measurements in 700 workplaces, supplemented by continuous radon measurements in 334 workplaces. The occupational radon concentration was calculated by multiplying the result of the integrated measurements by the seasonal correction factor and the ventilation correction factor (ratio between the working time and the full-time radon concentration obtained from continuous measurement). The annual radon concentration to which workers are exposed was weighted by the actual number of workers in each province. In addition, workers were divided into three main occupational categories (working mainly outdoors, underground, or indoors above ground). Probability distribution of the parameters affecting radon concentration levels were generated to calculate a probabilistic estimate of the number of workers exposed to excessive radon levels. With deterministic methods, the geometric and arithmetic mean radon concentrations in conventional, above-ground workplaces were 41 and 91 Bq m -3 , respectively. The estimated geometric and arithmetic mean annual radon concentrations that Finnish workers are exposed to were assessed as 19 and 33 Bq m -3 , respectively. The generic ventilation correction factor for workplaces was calculated as 0.87. Assessed with probabilistic methods, there are approximately 34,000 workers in Finland whose exposure to radon exceeds the reference level of 300 Bq m -3 . Although radon concentrations are generally low in Finnish workplaces, many workers are exposed to high levels of radon. Radon exposure in the workplace is the most common source of occupational radiation exposure in Finland.

Low-Level Radon Activity Concentration-A MetroRADON International Intercomparison.

An international comparison of continuous monitors measuring radon activity concentration was performed to validate the traceability of the European radon calibration facilities. It was carried out by comparing the secondary standards used by these previous facilities, ranging from 100 Bq·m-3 to 300 Bq·m-3. Secondary standards were individually compared to a secondary reference device previously calibrated in a reference radon atmosphere traceable to a primary standard. The intercomparison was organized by the National Institute for Nuclear, Chemical, and Biological Protection (SUJCHBO) in the period from October 2019 to April 2020 within the European Metrology Program for Innovation and Research (EMPIR), JRP-Contract 16ENV10 MetroRADON. Eight European laboratories participated in this study. The results of the experiment are presented and discussed.

The Metrological Traceability, Performance and Precision of European Radon Calibration Facilities.

An interlaboratory comparison for European radon calibration facilities was conducted to evaluate the establishment of a harmonized quality level for the activity concentration of radon in air and to demonstrate the performance of the facilities when calibrating measurement instruments for radon. Fifteen calibration facilities from 13 different European countries participated. They represented different levels in the metrological hierarchy: national metrology institutes and designated institutes, national authorities for radiation protection and participants from universities. The interlaboratory comparison was conducted by the German Federal Office for Radiation Protection (BfS) and took place from 2018 to 2020. Participants were requested to measure radon in atmospheres of their own facilities according to their own procedures and requirements for metrological traceability. A measurement device with suitable properties was used to determine the comparison values. The results of the comparison showed that the radon activity concentrations that were determined by European calibration facilities complying with metrological traceability requirements were consistent with each other and had common mean values. The deviations from these values were normally distributed. The range of variation of the common mean value was a measure of the degree of agreement between the participants. For exposures above 1000 Bq/m3, the variation was about 4% for a level of confidence of approximately 95% (k=2). For lower exposure levels, the variation increased to about 6%.

IMPROVING THE ASSESSMENT OF OCCUPATIONAL EXPOSURE TO RADON IN ABOVE-GROUND WORKPLACES.

Representative sampling of radon in indoor air is difficult because the concentration often exhibits unpredictable spatial and temporal variation. In workplaces, temporal variation may be rapid, and the minimum and maximum concentration can differ by a factor of 100. In this paper, we compare methods for assessing the radon concentration in workplaces utilising the results of an initial investigation with a track-etch detector and the results of an additional continuous measurement. The recommended method is as follows: the mean radon concentration during the working hours of 1 week, as well as the weekly mean, is calculated from the continuous measurement. The ratio between these mean concentrations is multiplied by the result from the track-etch detector. The coefficient of variation of this method is assessed as 19%. If the result of 1 week of continuous measurement is used alone, the coefficient of variation is assessed as 32%.

Radon in Finnish underground mines 2011-2019.

Radon measurements in Finnish underground mines were started in 1972. Since 1992, regular radon inspections by the competent authority have been carried out in all underground mines. During these inspections, several grab samples are taken from the air, which are later measured in the laboratory. This is a follow-up survey of radon concentrations in the air of the underground mines. The average radon concentrations in the mines between the years 2011 and 2019 varied from 90 to 1100 Bq m-3. Overall, the occupational radon exposure in the Finnish underground mines has remained at a low level from the 1990s onwards. In recent years, high radon concentrations have been observed only in those mines where active mining has ceased. Compared to other recent studies in mines in other countries, radon concentrations in Finnish mines are approximately at the same level. Uncertainties relating to infrequent grab sampling have been recognised and the authority is now testing personal radon detectors that may be used for the exposure assessment in the future.

210Pb and 210Po in Finnish cereals.

A survey was carried out on the activity concentrations of (210)Pb and (210)Po in cereal grains produced in Finland. The cereal species were wheat (Triticum aestivum), rye (Secale cereale), oats (Avena sativa) and barley (Hordeum vulgare), which account for 90% of the Finnish consumption of cereal products. The survey consisted of 18 flour and 13 unprocessed cereal samples and one hulled grain sample from 22 flour mills. According to the results, the mean (210)Pb/(210)Po concentrations in wheat grains, wheat flour, rye flour, oat grains and barley grains were 0.29, 0.12, 0.29, 0.36 and 0.36 Bq kg(-1), respectively. Combined with the consumption rates of the products, we assess that the mean effective doses from (210)Pb and (210)Po in cereal products for the adult male and female population are 22 and 17 µSv per year, respectively.

Prevention measures against radiation exposure to radon in well waters: analysis of the present situation in Finland.

Naturally occurring radioactive elements are found in all groundwaters, especially in bedrock waters. Exposure to these radioactive elements increases the risk of cancer. The most significant of these elements is radon which, as a gas, is mobile and dissolves in groundwater. In Finland, water supply plants are obliged to carry out statutory monitoring of the water quality, including radon. Monitoring of private wells, however, is often neglected. In this paper, we outline the problem by reviewing the outcomes of the studies conducted in Finland since the 1960s. We also summarise the development of legislation, regulations and political decisions made so far that have affected the amount of public exposure to radon in drinking water. A review of the studies on radon removal techniques is provided, together with newly obtained results. New data on the transfer of radon from water into indoor air are presented. The new assessments also take into account the expanding use of domestic radionuclide removal units by Finnish households.

Multidisciplinary analysis of Finnish esker sediment in radon source identification.

In order to define the naturally-occurring radioactive materials that are the source of radon in natural environments, a comprehensive analytical (geochemical, physical and chemical) methodology was employed to study sand samples from the Hollola esker in the city of Hollola (Lahti area, Finland). Techniques such as gamma-spectrometry, emanation measurements, sequential chemical extraction, scanning electron microscopy (SEM), electron probe microanalyses (EPMA) and inductively-coupled plasma mass spectrometry (ICP-MS) were used to determine the potential source of radon. Monazite and xenotime, uranium- and thorium-bearing minerals and potential radon sources, occurred in significant amounts in the samples and were also the main reason for the distribution of uranium and thereby radium in separate grain-size fractions. Following deposition, the esker sand has been exposed to no significant weathering, and radium has not therefore been much separated from uranium. However, considering its non-compatibility with crystal lattices, it was recognized rather in easily leachable species (44% of the total (226)Ra) than uranium (21% of the total (238)U) in our analyses. The smallest grain-size fraction of the esker sand had a higher emanation power (0.24) than the other fractions (around 0.17). Due to the small relative proportion of this fraction, however, it contributed only slightly to the total emanation (4%). The emanation power of the leachable species was about three times higher (ca. 0.20) than that of the species tightly bound to the crystal lattice (ca. 0.07).

Assessment of dose during the life cycle of natural stone production.

The environmental impact during the life cycle of natural stone production was studied. One of the points of interest was radiation. Natural stone samples from 23 quarries were surveyed for the radioactivity. One quarry was selected for a case study where the effective dose to the workers was assessed. The use of these stones in buildings was also evaluated with respect to the excess dose caused to the residents. According to the results the excess effective dose to the workers does not exceed 1 mSv a(-1) at the quarries. In buildings, all natural stones studied can be used safely as surfacing materials.